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To the 60-s test, VGs be upright making use of their heads flexing noted because of the reddish arrows inside Fig. Then, VGs drop off, and a lot of straighter and you can heavier graphite nanorods can be found in the brand new 90-s sample (Fig. 2D-2). Simultaneously, a good flake-for example diamond crystal (red photo inside the Fig. 2D-2) shows that diamond actually starts to appear, inside an excellent agreement for the SEM and you will Raman spectra. For the 120-s test, of numerous nanodiamond crystals naked to the edge of cauliflower-such as dust safeguarded the fresh graphite nanorods (Fig. 2E-2).

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To resolve this problem, we built a product to help you replicate it transition (Quand Appendix, Fig. S8). 4C implies that the fresh activation barrier of the O-ended system instead of tantalum atoms is 0.48 eV/unit cellphone, while it greatly reduces so you can −step three.99 eV/unit telephone on the Ta-additional O-ended system. This suggests one to O-ended system adsorbed by Ta atoms may also spontaneously changes to your diatomic coating diamond. The newest differential charges diagrams of the secret actions (0, 7, 8, and you can 9) (Fig. 4E and you may Quand Appendix, Fig. S9) intuitively reveal that each other Ta and you will O atoms sign up for the newest procedure of the fresh graphene stage transforming to your diamond. Furthermore, regarding the CVD system rather than a way to obtain Ta, hydrogen is the very important origin for the organization away from diamond. Which then shows that Ta are of higher benefit to the newest graphite-diamond stage conversion than simply H atoms.